I've finally looked into sorting out Wi-Fi syncing for my iPhone. I figured it would be a feature that was enabled by default, but it turns out it is not. Simple to solve though:
- Plug-in your device to your iTunes machine.
- Launch iTunes if it doesn't start automatically.
- Navigate to your device on the left-hand side.
- Make sure the summary tab is displayed.
- Click "Sync with this iPhone over Wi-Fi"

- Click the Sync button.


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